Brinkop , S. and Sausen , R . 1997 . A finite difference approximation for convective transports which maintains positive tracer concentrations . Beitr. Phys. Atmosph . 70 , 245 – 248 .
Broecker , W. , Peng , T.-H. , Ostlund , G. and Stuiver , M . 1985 . The distribution of bomb radiocarbon in the ocean . J. Geophys. Res . 90 , 6953 – 6970 .
Crutzen , P . 1976 . The possible importance of CSO for the sulfate layer of the stratosphere . Geophys. Res. Lett . 3 , 73 – 76 .
DeMore , W. B. , Sander , S. P. , Golden , D. M. , Hampson , R. F. , Kurylo , M. J. , Howard , C. J. , Ravishankara , A. R. , Kolb , C. E. and Molina , M. J . 1997 . Chemical kinetics and photochemical data for use in stratosphere modeling. Evaluation number 12. JPL publication 97-4, Jet Propulsion Laboratory, Pasadena, Calif., USA. Denning, A. S., Holzer, M., Gurney, K. R., Heimann, M., Law, R. M., Rayner, P. R., Fung, I. Y., Fan, S.-M., Taguchi, S., Friedlingstein, P., Balkanski, Y., Taylor, J., Maiss, M. and Levin, I. 1999. Three-dimensional transport and concentration of SF6: a model intercomparison study (Transcom 2) . Tellus 51 , 266 – 297 .
Elkins , J. W. , Fahey , D. W. , Gilligan , J. M. , Dutton , G. S. , Baring , T. J. , Volk , C. M. , Dunn , R. E. , Myers , R. C. , Montzka , S. A. , Wamsley , P. R. , Hayden , A. H. , Butler , J. H. , Thompson , T. M. , Swanson , T. H. , Dlugokencky , E. J. , Novelli , P. C. , Hurst , D. F. , Lobert , J. M. , Ciciora , S. J. , McLaughlin , R. J. , Thompson , T. L. , Winkler , R. H. , Fraser , P. J. , Steele , L. D. and Lucarelli , M. P . 1996 . Airborne gas chromatograph for in situ measurements of long-lived species in the upper troposphere and lower stratosphere . Geophys. Res. Lett . 23 , 347 – 350 .
Feichter , J. and Crutzen , P. J . 1990 . Parameterization of vertical transport due to deep cumulus convection in a global transport model and its evaluation with 'Radon measurements . Tellus 42 , 100 – 117 .
Geller , L. S. , Elkins , J. W. , Lobert , J. M. , Clarke , A. D. , Hurst , D. F. , Butler , J. H. and Myers , R. C . 1997 . Tropospheric SF6: observed latitudinal distribution and trends, derived emissions and interhemispheric exchange time . Geophys. Res. Lett . 24 , 675 – 678 .
Grewe , V. and Dameris , M . 1996 . The large-scale mass-exchange between stratosphere and troposphere in the ECHAM3 model . In Staniforth , A. (ed.) : Research activities in atmospheric and oceanic modelling. CAS/ JSC working group on numerical experimentation. Report No. 23 WMO/TD No. 734.721-722 , Geneva , Switzerland .
Hall , T. M. and Plumb , R. A . 1994 . Age as a diagnostic of stratospheric transport . J. Geophys. Res . 99 , 1059 – 1070 .
Harnisch , J. , Borchers , R. , Fabian , P. and Maiss , M . 1996 . Tropospheric trends for CF4 and C2F6 since 1982 derived from SF6 dated stratospheric air . Geo-phys. Res. Lett . 23 , 1099 – 1102 .
Hesshaimer , V. , Heimann , M. and Levin , I . 1994 . Radiocarbon evidence for a smaller oceanic carbon dioxide sink than previously believed . Nature 370 , 201 – 203 .
Holton , J. R. , Haynes , P. H. , McIntyre , M. E. , Douglas , A. R. , Rood , R. B. and Pfister , L. , 1995 . Stratosphere-troposphere exchange . Rev. Geophys . 33 , 403 – 439 .
Jacob , D. J. , Prather , M. J. , Wofsy , S. C. and McElroy , M. B . 1987 . Atmospheric distribution of “Kr simulated with a general circulation model . J. Geophys. Res . 92 , 6614 – 6626 .
Jacob , D. J. , Prather , M. J. , Rasch , P. J. , Shia , R.-L. , Balkanski , Y. J. , Beagley , S. R. , Bergmann , D. J. , Black-shear , W. T. , Brown , M. , Chiba , M. , Chipperfield , M. P. , de Grandpré , J. , Dignon , J. E. , Feichter , J. , Genthon , C. , Grose , W. L. , Kasibathla , P. S. , Kohler , I. , Kritz , M. A. , Law , K. , Penner , J. E. , Ramonet , M. , Reeves , C. E. , Rotman , D. A. , Stockwell , D. Z. , van Velthoven , P. F. J. , Verver , G. , Wild , O. , Yang , H. and Zimmermann , P . 1997 . Evaluation and intercomparison of global atmospheric transport models using 222Rn and other short-lived tracers . J. Geophys. Res . 102 , 5953 – 5970 .
Johnston , H . 1989 . Evaluation of excess carbon 14 and strontium 90 data for suitability to test two-dimensional stratospheric models . J. Geophys. Res . 94 , 18485 – 18493 .
Kentarchos , A. S. , Roelofs , G. J. and Lelieveld , J . 1999 . Model study of a stratospheric intrusion event at lower midlatitudes associated with the development of a cutoff low . J. Geophys. Res . 104 , 1717 – 1727 .
Kjellstrom , E . 1998 . A three-dimensional global model study of carbonyl sulfide in the troposphere and the lower stratosphere . J. Atmos. Chem . 29 , 151 – 172 .
Land , C . 1999. Untersuchungen zum globalen Spuren-stofftransport mit dem Atmosphaerenmodell ECH-AM4.L39(DLR). PhD Thesis, University of Munich , Germany.
Leifer , R . 1992 . Project AIRSTREAM: Trace gas final report. USDOE Report EML-549, New York, USA. Levin, I. and Hesshaimer, V. 1996. Refining of atmospheric transport model entries by the globally observed passive tracer distributions of “Kr and sulfur hexafluoride (SF6) . J. Geophys. Res . 101 , 16745 – 16755 .
Maiss , M. and Levin , I . 1994 . Global increase of SF6 observed in the atmosphere . Geophys. Res. Lett . 21 , 569 – 572 .
Maiss , M. , Steele , P. , Francey , R. J. , Fraser , P. J. , Langen-felds , R. L. , Trivett , N. B. A. and Levin , I . 1996 . Sulfur hexafluoride - a powerful new atmospheric tracer . Atmos. Environ . 30 , 1621 – 1629 .
Maiss , M. and Brenninkmeijer , C. A. M . 1998 . Atmo-spheric SF6 trends, sources and prospects . Environ. Sci. Technol . 32 , 3077 – 3086 .
Nydal , R. and Lovseth , K . 1983 . Tracing bomb 1-4C in the atmosphere 1962-1980 . J. Geophys. Res . 88 , 3621 – 3642 .
Nydal , R. and Lovseth , K . 1996. Carbon-14 measurements in atmospheric CO2 from northern and southern hemi-sphere sites , 1962-1993. ORNL/CDIAC-93, NDP-057. Carbon Dioxide information analysis center , Oak Ridge National Laboratory , Oak Ridge, Tennessee, USA , 67 pp.
Oeschger , H. , Siegenthaler , U. , Schotterer , U. and Gugel-mann , A . 1975 . A box diffusion model to study the carbon dioxide exchange in nature . Tellus 27 , 168 – 192 .
Patra , P. K. , Lal , S. , Subbaraya , B. H. , Jackman , C. H. and Rajaratnam , P . 1997 . Observed vertical profile of sulphur hexafluoride (SF6) and its atmospheric applications . J. Geophys. Res . 102 , 8855 – 8859 .
Prather , M. , McElroy , M. , Wofsy , S. , Russell , G. and Rind , D . 1987 . Chemistry of the global troposphere: Fluorocarbons as tracers of air motions . J. Geophys. Res . 92 , 6579 – 6613 .
Rasch , P. and Williamson , D . 1990 . Computational aspects of moisture transport in global models of the atmosphere . Q. J. R. Meteorol. Soc . 116 , 1071 – 1090 .
Ravishankara , A. R. , Solomon , S. , Turnipseed , A. A. and Warren , R. F . 1993 . Atmospheric lifetimes of long-lived halogenated species . Science 259 , 194 – 199 .
Roeckner , E. , Arpe , K. , Bengtsson , L. , Christoph , M. , Claussen , M. , Dflmenil , L. , Esch , M. , Giorgetta , M. , Schlese , U. and Schulzweida , U . 1996 . The atmospheric general circulation model ECHAM-4: Model descrip-tion and simulation of present-day climate. Report no. 218 , Max-Planck-Institute for Meteorology , Hamburg , Germany .
Roelofs , G. and Lelieveld , J . 1995 . Distribution and budget of 03 in the troposphere calculated with a chemistry general circulation model . J. Geophys. Res . 100 , 20983 – 20998 .
Rosenlof , K. and Holton , J . 1993 . Estimates of the strato-spheric residual circulation using the downward control principle . J. Geophys. Res . 98 , 10465 – 10479 .
Siegenthaler , U . 1983 . Uptake of excess CO2 by an out-crop-diffusion model of the ocean . J. Geophys. Res . 88 , 3599 – 3608 .
Siegmund , P. C. , van Velthoven , P. F. J. and Kelder , H. , 1996 . Cross-tropopause transport in the extratropical northern winter hemisphere diagnosed from high- resolution ECMWF data . Q. J. R. Meteorol. Soc . 122 , 1921 – 1941 .
Song , N. , Starr , D. , Wuebbles , D. , Williams , A. and Larson , S . 1996 . Volcanic aerosols and interannual variation of high clouds . Geophys. Res. Lett . 23 , 2657 – 2660 .
Steil , B. , Dameris , M. , Brühl , C. , Crutzen , P. J. , Grewe , V. , Ponater , M. and Sausen , R . 1997 . Development of a chemistry module for GCMs: First results of a multiannual integration . Annales Geophysical 16 , 205 – 228 .
Stuiver , M . 1980 . 1-4C distribution in the Atlantic Ocean . J. Geophys. Res . 85 , 2711 – 2718 .
Stuiver , M. , Ostlund , H. G. and McConnaughey , T. A. 1981. GEOSECS Atlantic and Pacific 1-4C distribution. In: Carbon cycle modelling, B. Bolin (ed.) John Wiley, New York, USA, pp. 201 – 221
Telegadas , K . 1971. The seasonal stratospheric distribu-tion and inventory of carbon-14 from March 1955 to July 1969. Health and Safety Lab, U.S. Atomic Energy Comm., Washington, DC, USA, Report 243.
Telegadas , K. , Gray , J. , Sowl , R. E. and Ashenfelter , T. E . 1972. Carbon-14 measurements in the stratosphere from a balloon-borne molecular sieve sampler, Health and
Safety Lab ., US Atomic Energy Comm. , Washington, DC, USA , report 246.
Tiedtke , M . 1989 . A comprehensive mass flux scheme for cumulus parameterization in large-scale models. Mon . Wea. Re v . 117 , 1779 – 1800 .
Wang , Y. , Jacob , D. J. and Logan , J. A . 1998 . Global simulation of tropospheric 03-hydrocarbonchemistry (3). Origin of tropospheric 03 and effects of nonmethane hydrocarbons . J. Geophys. Res . 103 , 10757 – 10767 .
Waugh , D. W. , Hall , T. M. , Randel , W. J. , Rasch , P. J. , Boville , B. A. , Boering , K. A. , Wofsy , S. C. , Daube , B. C. , Elkins , J. W. , Fahey , D. W. , Dutton , G. S. , Volk , C. M. and Vohralik , P. F . 1997 . Three-dimensional simulations of long-lived tracers using winds from MACCM2 . J. Geophys. Res . 102 , 21493 – 21513 .
World Meteorological Organization (WMO) . 1994. Scientific assessment of ozone depletion. Report 37, Global ozone research and monitoring project. Geneva, Switzerland.
World Meteorological Organization (WMO) . 1986. Atmospheric ozone 1985: Report 16, Global ozone research and monitoring project. Geneva, Switzerland.