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Original Research Papers

Atmospheric new particle formation at Utö, Baltic Sea 2003–2005

Authors:

A. -P. Hyvärinen ,

Finnish Meteorological Institute, Research and Development, FI
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M. Komppula,

Finnish Meteorological Institute, Research and Development, FI
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C. Engler,

Finnish Meteorological Institute, Research and Development, FI; Institute for Tropospheric Research, Department of Physics
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N. Kivekäs,

Finnish Meteorological Institute, Research and Development, FI
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V. -M. Kerminen,

Finnish Meteorological Institute, Research and Development, FI
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M. Dal Maso,

Department of Physical Sciences, University of Helsinki, FI; Research Center Jülich GmbH, DE
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Y. Viisanen,

Finnish Meteorological Institute, Research and Development, FI
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H. Lihavainen

Finnish Meteorological Institute, Research and Development, FI
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Abstract

Nearly 3 yr (March 2003–December 2005) of continuous particle number size distribution measurements have been conducted at the island of Utö in the Baltic Sea. The measured particle size range was from 7 to 530 nm. During the measurement period, a total of 103 regional new-particle formation events were observed. The characteristics of the nucleation events at Utö were similar to those reported in the literature in other Nordic sites, though measured condensation sinks were rather high (geometric mean of 3.8 × 10-3 s-1) during event days. Clear evidence was found that new particles nucleate regionally near Utö, rather than are transported from greater distances. However, the Baltic Sea seems to have an inhibiting effect on new-particle formation. The boreal forest areas in the continental Finland were found to have an enhancing effect on the nucleation probability in Utö, suggesting that at least some of the precursor gases for nucleation and/or condensational growth of particles originate from these forests. In addition to regional new-particle formation events, a total of 94 local events were observed in Utö. These are short-lived events with a small footprint area, and can at least partly be tracked down to the emissions of ship traffic operating at Utö.

How to Cite: Hyvärinen, A.-P., Komppula, M., Engler, C., Kivekäs, N., Kerminen, V.-M., Maso, M.D., Viisanen, Y. and Lihavainen, H., 2008. Atmospheric new particle formation at Utö, Baltic Sea 2003–2005. Tellus B: Chemical and Physical Meteorology, 60(3), pp.345–352. DOI: http://doi.org/10.1111/j.1600-0889.2008.00343.x
  Published on 01 Jan 2008
 Accepted on 14 Feb 2008            Submitted on 11 Oct 2007

References

  1. Birmili , W. , Wiedensohler , A. , Heintzenberg , J. and Lehmann , K . 2001 . Atmospheric particle number size distribution in central Europe: sta-tistical relations to air masses and meteorology. J. Geophys. Res . 106 , 32005 – 32018 .  

  2. Boy , M. , Kulmala , M. , Ruuskanen , T. M. , Pihlatie , M. , Reissell , A. , and co-authors . 2005 . Sulphuric acid closure and contribution to nucle-ation mode particle growth. Atmos. Chem. Phys . 5 , 863 - 878 .  

  3. Dal Maso , M. , Kulmala , M. , Riipinen , I., Wagner, R., Hussein, T., and co-authors. 2005. Formation and growth of fresh atmospheric aerosols: eight years of aerosol size distribution data from SMEAR II, Hyytiälä, Finland. Boreal Environ. Res . 10 , 323 - 336 .  

  4. Dal Maso , M. , Sogacheva , L. , Aalto , P. P. , Riipinen , I., Komppula, M., and co-authors. 2007. Aerosol size distribution measurements at four Nordic field stations: identification, analysis and trajectory analysis of new particle formation bursts. Tellus 59B , 350 - 361 .  

  5. Devasthale , A ., Kröger , O . and Grassl , H . 2006 . Impact of ship emissions on cloud properties over coastal areas . Geophys. Res. Lett . 33 , L02811, doi: https://doi.org/10.1029/2005GL024470 .  

  6. Durkee , P. A. , Noone , K. J. and Bluth , R. T . 2000 . The monterey area ship track experiment. J. Atmos. Sci . 57 , 2523 – 2541 .  

  7. Engler , C. , Lihavainen , H. , Komppula , M. , Kerminen , V.-M. , Kulmala , M. , and co-authors . 2007 . Continous measurements of aerosol prop-erties at the Baltic Sea. Tellus 59B , 728 - 741 .  

  8. Hobbs , P. V. , Garret , T. J. , Ferek , R. J. , Strader , S. R. , Hegg , D. A. , and co-authors . 2000 . Emissions from ships with respect to their effects on clouds. J. Atmos. Sci . 57 ( 16 ), 2570-2590 .  

  9. Hyvönen , S. , Junninen , H. , Laakso , L. , Dal Maso , M. , Grönholm , T. , and co-authors . 2005 . A look at aerosol formation using data mining techniques. Atmos. Chem. Phys . 5 , 3345 - 3356 .  

  10. Kerminen , V.-M. , Lihavainen , H. , Komppula , M. , Viisanen , Y. and Kulmala , M . 2005 . Direct observational evidence linking atmospheric aerosol formation and cloud droplet activation. Geophys. Res. Lett . 32 , L14803 , doi: https://doi.org/10.1029/2005GL023130 .  

  11. Kittelson , D. B. , Watts , W. E and Johnson , J. P . 2006 . On-road and lab-oratory evaluation of combustion aerosols—Part 1: summary of diesel engine results. J. Aerosol Sci . 37 , 913 – 930 .  

  12. Komppula , M. , Lihavainen , H. , Hatakka , J. , Paatero , J. , Aalto , P. , and co-authors . 2003a . Observations of new particle formation and size distribution at two different heights and surroundings in subarctic area in northern Finland./. Geophys. Res . 108 ,4295-4306.  

  13. Komppula , M. , Dal Maso , M. , Lihavainen , H. , Aalto , P. , Kulmala , M. , and co-authors . 2003b . Comparison of new particle formation events at two locations in northern Finland. Boreal Environ. Res . 8 ,395-404. Kristensson, A., Dal Maso, M., Swietlicki, E., Hussein, T., Zhou, J., and co-authors. 2008. Characterization of New Particle Formation Events at a B ackground Site in Southern Sweden: relation to Air Mass History. Tellus 60B, this issue.  

  14. Kulmala , M. , Hämeri , K. , Aalto , P. P. , Maela , J. M. , Pirjola , L. , and co-authors . 2001a . Overview of the international project on biogenic aerosol formation in the boreal forest (BIOFOR). Tellus 53B , 324 - 343 .  

  15. Kulmala , M. , Dal Maso , M. , Mäkelä , J. M. , Pirjola , L. , Väkevä , M. , and co-authors . 2001b . On the formation growth and composition of nucleation mode particles . Tellus 53B , 479 - 490 .  

  16. Kulmala , M. , Vehkamai , H. , Petäjä , T. , Dal Maso , M. , Lauri , A. , and co-authors . 2004 . Formation and growth rates of ultrafine atmospheric particles: a review of observations. J. Aerosol Sci . 35 ,143-176.  

  17. Laaksonen , A. , Hamed , A. , Joutsensaari , J. , Hiltunen , L. , Cavalli , E , and co-authors . 2005 . Cloud condensation nucleus production from nucleation events at a highly polluted region. Geophys. Res. Lett . 32 , L06812, doi: https://doi.org/10.1029/2004GL022092 .  

  18. Lihavainen , H. , Kerminen , V.-M. , Komppula , M. , Hatakka , J. , Aaltonen , V. , and co-authors . 2003 . Production of “potential” cloud condensation nuclei associated with atmospheric new—particle for-mation in northern Finland. J. Geophys. Res . 108(D24), 4782, doi: https://doi.org/10.1029/2003JD003887 .  

  19. Mäkelä , J. M. , Koponen , I. K. , Aalto , P. and Kulmala , M . 2000 . One-year data of submicron size modes of tropospheric background aerosol in southern Finland. J. Aerosol. Sci . 31 , 595 – 611 .  

  20. Rohrer , E and Berresheim , H . 2006 . Strong correlation between levels of troposheric hydroxyl radicals and solar ultraviolet radiation. Nature 442 , 184 – 187 .  

  21. Russell , L. M. , Seinfeld , J. H. , Flagan , R. C. , Ferek , R. J. , Hegg , D. A. , and co-authors. 1999 . Aerosol dynamics in ship tracks . J. Geophys. Res . 104 ,31077-31095.  

  22. Rönkko , T. , Virtanen , A. , Vaaraslahti , K. , Keskinen , J. , Pirjola , L . and Lappi , M . 2006 . Effect of dilution conditions and driving parameters on nucleation mode particles in diesel exhaust: laboratory and on-road study . Atmos. Environ . 40 , 2893 - 2901 .  

  23. Scheier , M. , Kokhanovsky , A. A. , Euring , V. , Bugliaro , L. , Mannstein , H. , and co-authors . 2006 . Impact of ship emissions on the microphys-ical, optical and radiative properties of marine stratus: a case study. Atmos. Chem. Phys . 6 ,4925-4942.  

  24. Sciare , J. , Bardouki , H. , Moulin , C . and Mihalopoulos , N . 2003 . Aerosol sources and their contribution to the chemical composition of aerosols in the Eastern Mediterranean Sea during summertime. Atm. Chem. Phys . 3 ,291-302.  

  25. Sogacheva , L. , Dal Maso , M. , Kerminen , V.-M. and Kulmala , M . 2005 . Probability of nucleation events and aerosol particle concentrations in different air mass types arriving at Hyytiälä, Southern Finland, based on back trajectories analysis. Boreal Environ. Res . 10, 479 – 491 .  

  26. Spracklen , D. V. , Carslaw , K. S. , Kulmala , M. , Kerminen , V.-M. , Mann , G. W. , and co-authors . 2006 . The contribution of boundary layer nu-cleation events to total particle concentrations on regional and global scales. Atmos. Chem. Phys . 6 ,5631-5648.  

  27. Stohl , A. , Wotawa , G. , Seibert , P. and Kromp-Kolb , H . 1995 . Interpola-tion errors in wind fields as a function of spatial and temporal reso-lution and their impact on different types of kinematic trajectories. J. Appl. Meteorol . 34 , 2149 – 2165 .  

  28. Svenningsson , B. , Ameth , A. , Hayward , S. , Holst , T. , Massling , A , and co-authors . 2008 . Aerosol particle formation events and analysis of high growth rates observed above a subarctic wetland-forest mosaic. Tellus 60B , this issue.  

  29. Tunved , P. , Nilsson , E. D. , Hansson , H.-C. , Strom , J. , Kulmala , M. , and co-authors. 2005 . Aerosol characteristics of air masses in northern Europe: influences of location, transport, sinks, and sources . J. Geophys. Res . 110 , D07201.  

  30. Tunved , P. , Hansson , H.-C. , Kerminen , V.-M. , Strom , J. , Dal Maso , M. , and co-authors. 2006 . High natural aerosol loading over boreal forests . Science 312 (5771) , 261 - 263 .  

  31. Vehkamäki , H. , Dal Maso , M. , Hussein , T. , Flanagan , R. , Hyvärinen , A. , and co-authors. 2004 . Atmospheric particle formation events at Värrio measurement station in Finnish Lapland 1998-2002. Atmos. Chem. Phys . 4 , 2015– 2023 .  

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